Professional Documents
Culture Documents
National Engineering School of Monastir, Unit of Thermic and Thermodynamics of the Industrial Processes, Avenue Ibn El Jazzar, 5019 Monastir, Tunisia
Aix Marseille Universit, CNRS, IUSTI UMR 7343, 13453 Marseille, France
a r t i c l e
i n f o
Article history:
Received 2 May 2013
Received in revised form 18 June 2014
Accepted 26 June 2014
Available online 9 July 2014
Keywords:
Turbulent uidization
CFD
Drag model
Turbulence
Wall boundary conditions
a b s t r a c t
A numerical study was carried out to explore the hydrodynamic behavior of gassolid ow in a 2D turbulent uidized bed. The gassolid ow was simulated by mean of an EulerianEulerian two uid model
incorporating the Kinetic Theory of Granular Flow (KTGF). The main purpose of this work was to examine
the ability of various models to predict the hydrodynamic of a turbulent uidized bed lled with Geldart
B particles on the Fluent V.6.2 platform. The effect of different drag models including those of Gidaspow,
Syamlal & OBrien and Mckeen, were tested and the corresponding results were compared. A good level of
agreement was achieved with the Gidaspow model with reference to experimental data. Two viscous
models were tested and the standard ke model performed the better prediction of the core annular
structure of the bed with reference to the experimental data. Different wall boundary conditions were
also tested and their impact evaluated on the hydrodynamics of the bed.
2014 The Society of Powder Technology Japan. Published by Elsevier B.V. and The Society of Powder
Technology Japan. All rights reserved.
1. Introduction
The turbulent uidized bed was widely used in industrial applications during the last decades. It is characterized by its ability to
handle the continuous powder, its vigorous gassolids contacting,
its ability of favorable heat and mass transfer and by its relatively
low axial gas dispersion.
The turbulent uidization regime has been commonly acknowledged as a distinct ow regime occurring between two adjacent
ow regimes: the bubbling and the fast uidization regimes. It is
characterized by two different coexisting regions: a dense bottom,
bubbling region and a dilute, dispersed ow region. The turbulent
uidization is further characterized by its high value of dispersion
coefcient for the solids. According to the literature review, less
attention was dedicated to the turbulent uidization due to current deciencies in experimental and theoretical works [14].
Therefore, fundamental understanding of its hydrodynamic behavior is required.
Having achieved success in simulation of single phase ow, Computational Fluid Dynamics (CFD) is considered greatly promising for
modeling multiphase ows [5]. Nevertheless, CFD is still at the verication and validation stages for modeling multiphase ows, for
uidized bed applications particularly, and more improvements
http://dx.doi.org/10.1016/j.apt.2014.06.024
0921-8831/ 2014 The Society of Powder Technology Japan. Published by Elsevier B.V. and The Society of Powder Technology Japan. All rights reserved.
1738
Nomenclature
C 2e , C 1e
CD
D
ds
es
g
g0
Gk;g
Gs
H
I
I2D
J
kg
kH
P
Ps
q
Re
t
u
udr
Ug
Greek letters
eg
turbulence dissipation of gas phase, m2 s3
a
volume fraction
q
density, kg m3
ns
solid bulk viscosity, Pa s
u
specularity coefcient
rk ; re
turbulent Prandtl numbers
b
gasparticle interaction coefcient, kg m3 s1
H
granular temperature, m2 s2
s
stress tensor, N m2
/
angle of internal friction,
Pkg ; Pg inuence of the dispersed phases on the continuous
phase
c
collisional dissipation of energy, kg m3 s1
Subscripts
KTGF
Kinetic Theory of Granular Flow
Col
collisional
Kin
kinetic
max
maximum
fr
frictional
X
lateral coordinate, m
s
solid phase
g
gas phase
model with a scaling factor C varying between 0.2 and 0.3. The correction factor of 0.25 proved to predict the experimental results
observed in a freely bubbling bed for FCC with a mean diameter
of (75 lm).
Yang et al. [26] adopted the energy minimization multiscale
(EMMS) approach, proposed by Li and Kwauk [27] to calculate the
drag coefcient from structure parameters, and to incorporate it
into the two uid models. They claimed that this approach reasonably resolves the heterogeneous structures and suggested the feasibility of using it as a sub-grid closure law for the drag coefcient.
More recently, the EMMS drag model was applied by Jiradilok
et al. [2] to predict the hydrodynamic of the turbulent uidization
of FCC particles. They found that the turbulent regime was correctly computed using the modied drag of Yang et al. [26].
Although several correlations exist in the literature for the drag
force, considerable uncertainties still remain for its prediction.
In addition to the drag coefcient, the restitution coefcient
which accounts for the inelasticity of the particleparticle collision
may affect the hydrodynamic of a uidized bed. Indeed, being an
input in the kinetic theory based CFD models, it has a direct impact
on the quantities they contain, such as particle pressure, particle
viscosity and dissipation of particle temperature. Goldschmidt
et al. [10], studied the effect of the restitution coefcient on the
hydrodynamic of a dense gas uidized bed. They reported that, to
obtain realistic simulations using fundamental hydrodynamic models, it is important to correctly take the effect of non-ideal particle
particle encounters into account. Taghipour et al. [28] found higher
sensitivity to the restitution coefcient at U < U mf . Gao et al. [29]
indicated that there is sensitivity to this coefcient in the behavior
of a turbulent bed lled with Geladart B particles when its values
range from 0.6 to 0.99. Although, the effect of the restitution coefcient has been extensively explored, the role of this parameter is not
yet fully understood and more explorations are still required.
In the riser of a turbulent uidized bed, the multiphase ow is
very turbulent and displays high Reynolds numbers. In order to
make the simulation predictions more realistic, the time average
turbulent behavior and the turbulent interaction between phases
1739
should be taken into account. Different models, laminar and turbulent models with kinetic theory, have been used by various authors
to simulate the hydrodynamic of gasparticle multiphase ow.
Almuttahar and Taghipour [30] compared two different viscous
models, the ke turbulence and the laminar model with Kinetic
Theory of Granular Flow. They claimed that the laminar model predictions give more consistent results than the turbulent models.
Nevertheless, this comparison was carried out in 2D modeling
and since turbulence uctuations always have three-dimensional
spatial character then, to draw a rm conclusion, 3D comparative
studies are required. However, this requires excessive computational time, hence the 2D modeling still takes preference over 3D.
Further parameters may affect the simulation results of a turbulent uidized bed, such as the wall boundary conditions. Li et al.
[31] investigated the impact of this parameter in a 2D simulation
of a bubbling uidized bed, for gas and solid phases, over the generated ow hydrodynamics. According to their investigation, the
wall boundary conditions need to be specied with great care
due to their high relevance over the hydrodynamic. Johnson and
Jackson [32] have developed a set of boundary conditions to dene
the interactions between the particles and the wall. These boundary conditions have been widely applied in numerical simulations
of gassolid ows due to their relatively simple form [29,33]. In
Johnson and Jackson boundary conditions, the specularity coefcient, which characterizes the tangential momentum transfer due
to collision between the particles and the wall, must be specied
with great care as well (Li et al. [31]). The effect of this coefcient
on the numerical results for different solid particle distributions
has been studied by several researchers [31,34]. The core-annulus
structure of the solid phase was reported to be very sensitive to the
choice of the specularity coefcient [31,35,36]. However, choosing
the right number is critical for most validation studies due to the
difculty in measurements. Further theoretical investigations are
then required in order to contribute to a better understanding of
the gassolid ows.
Cyclone
Flow meter
Riser
PDA
Valve
Buffer vessel
Pump
Air outlet
D
Lifting screw
Y
Air distributor
Air inlet
Fig. 1. Schematic of the experimental apparatus of the turbulent uidized bed.
1740
Table 1
Governing equations.
Equations
Mathematical expressions
@ag qg
r g g~
ug 0
@t
@as qs
~
r
u
s
s 0
s
@t
(T1-1)
aq
aq
(T1-2)
ag + as = 1
ug
@ag qg ~
!!
r g g~
ug ~
ug r g g rP b ug us g g g
@t
!
!
us
@as qs ~
r s s~
us~
us r g s rP b ug us s s g
@t
1 02
H 3u
3 @as qs H
r s s~
us H P sI s : r~
us r q J
@t
2
aq
aq
Granular Temperature
Equation of conservation of solids uctuating energy
aq
aq
s : r~
us c
0 P sI s
aq
(T1-3)
(T1-4)
(T1-5)
(T1-6)
(T1-7)
(T1-8)
Table 2
Constitutive equations.
Equations
Gas phase stress tensor (Lun et al. [41])
Solid phase stress tensor (Lun et al. [41])
Solids pressure (Lun et al. [41])
Solids shear viscosity
Collisional viscosity (Gidaspow et al. [14])
Kinetic viscosity (Gidaspow et al. [14])
Kinetic viscosity (Syamlal et al. [18])
Frictional viscosity (Schaeffer et al. [40]
Mathematical expressions
h
i
T
sg ag ng 23 lg r ~
ug I lg r~
ug r~
ug
h
i
T
ss as ns 23 ls r ~
us I ls r~
us r~
us
P s as qs H
a qs H1 es
ls = ls,col + ls,kin + ls,fr
p
(T2-4)
(T2-5)
2
qs ds
4
ls;kin 10
96 Hp 1es as g 0 1 5 g 0 as 1 es
p
as qs ds Hp
ls;kin 63es
/
ls;fr P2spsin
I
2
5 g0
(T2-2)
(T2-3)
2g 0 2s
ls;col 45 as qs ds g 0 1 es
(T2-1)
as 1 es 3es 1
(T2-6)
(T2-7)
(T2-8)
2D
q
ns 43 as qs ds g 0 1 es H
p
1=3 1
a
s
g 0 1 as;max
q
cs 31 e2s a2s qs g 0 H d4p Hp
(T2-9)
(T2-10)
(T2-11)
1741
Mathematical expressions
ag > 0.8
b 34 C D0
(T3-1)
ag 1ag
qg j~
ug ~
us ja2:65
ds
ag 6 0.8
(T3-2)
2
q
1a lg
1:751 ag dgs j~
ug ~
us j
b 150 ag g
ds 2
0:687
24
1
0:15Re
;
Re
<
1000
s
s
Re
s
C D0
0:44;
Res > 1000
(T3-3)
Res
(T3-4)
!
b 4 #2 d C D jus ug j
r;s s
2
4:8
C D 0:63 p
(T3-5)
ag qg j~
ug ~
us jds
lg
!
3 as ag qg
(T3-6)
Res =#r;s
q
#r;s 0:5A 0:06Res 0:06Res 2 0:12Res 2B A A2
8 1:28
ag 6 0:85
< P ag
Q
;
B
A a4:14
ag > 0:85
g
: ag
Mckeen drag model [24]
(T3-7)
(T3-8)
P = 0.8 et Q = 2.65
!
q j!
g u s ug j
as ag1:8
b C 17:3
Res 0:336
ds
(T3-9)
The Reynolds stress tensor for the gas phase, given in Eq. (T1-7),
takes the following form:
2
3
!
where U g denotes the gas-weighted velocity and lt;g is the gas turbulent viscosity given by the following expression:
lt;g qg C l
kg
eg
lt;g
!
@
ag qg kg r ag qg U g kg r ag
rk ag Gk;g
@t
rk g
ag qg eg ag qg Pkg
lt;g
!
@
e
ag qg eg r ag qg U g eg r ag
re ag g
@t
re g
kg
C 1e Gk;g C 2e qg eg
ag qg Peg
where Pkg and Peg represent the inuence of the dispersed phases
on the continuous phase and Gk;g the production of turbulent kinetic
energy. These terms are given by the following equations:
Pkg
ag qg
Peg C 3e
ksg 2kg ~
ugs ~
udr
eg
kg
Pkg
ug r~
ug : r~
ug
Gk;g lt;g r~
1742
Table 4
Modeling parameters.
Description
Riser height H
Riser width
Static bed height H0
Gas density qg
Particle density qs
Particle diameter ds
Initial solid volume fraction a0
Inlet gas velocity Ug
Solid ux Gs
Angle of internal friction
Restitution coefcient es
Specularity coefcient u
Maximum particle packing limit
Time step
Value
2m
0.2 m
0.1 m
1.2 kg/m3
2400 kg/m3
120 lm
0.6
0.9 m/s, 1 m/s, 1.1 m/s
0.1 kg/m2s, 0.22 kg/m2s, 0.413 kg/m2s
30
0.8, 0.9, 0.95 and 0.99
0, 0.001, 0.25 and 1
0.64
103 s
0
0.5
0.6
0.7
0.8
0.9
(X/D)
-1
Gidaspow
Syamlal
-2
Mckeen
Exp (Van Den Moortel, 1998)
-3
Fig. 3. The time-averaged axial particle velocity predicted along the radial direction
by various drag models at Y 1 m (supercial gas velocity U g 1 m=s, ke
turbulent model, es 0:9, u 1).
1743
0
0.5
0.6
0.7
0.8
0.9
(X/D)
Gidaspow
-1
Syamlal
Mckeen
Exp (Van Den Moortel, 1998)
-2
Fig. 4. The time-averaged axial particle velocity predicted along the radial direction
by various drag models at Y 1:2 m (supercial gas velocity U g 1 m=s, ke
turbulent model, es 0:9, u 1).
that the Mckeen drag model cannot capture the dilute characteristics of turbulent uidized beds in spite of the better prediction for
the dense region.
Gidaspow drag model provided good description of the hydrodynamic of uidized beds lled with Geldart B particles (Lu et al.
[53]). In the present work, the same model gave reasonable qualitative and quantitative agreement with reference to experimental
data in term of particle velocity proles. We propose then to adopt
the Gidaspow drag model in the rest of this work.
5.1.2. Comparison of the laminar and the turbulence model
To study the effect of turbulence modeling on ow predictions,
simulations with laminar model and ke turbulent model were
conducted and further compared to experimental measurements.
Fig. 5 compares the time averaged axial solid velocity obtained
with both models to experimental data evaluated at Y 1:2 m.
In both models, the core-annulus structure of the gassolid ow
is well predicted. However, the solid velocity prole predicted by
the standard ke model provides a better agreement with the
0
0.5
0.6
0.7
0.8
0.9
(X/D)
-1
Turbulent
Laminar
Exp (Van Den Moortel, 1998)
-2
Fig. 5. The time-averaged axial particle velocity predicted along the radial direction
by laminar and turbulent model at Y 1:2 m (supercial gas velocity U g 1 m=s,
Gidaspow drag model, es 0:9, u 1).
Fig. 6. The computed instantaneous solid volume fraction for three different
restitution coefcient at t 30 s (supercial gas velocity U g 1 m=s, Gidaspow
drag model, ke turbulent model, u 1).
1744
0
0.5
0.6
0.7
0.8
0.9
(X/D)
Rest. 0.8
-1
Rest. 0.9
0
0.5
0.6
0.7
0.8
0.9
(X/D)
-1
Spec.coeff=0
Spec.coeff=0.001
Rest. 0.95
Spec.coeff =0.25
Rest. 0.99
Spec.coeff=1
-2
-2
Fig. 7. The time-averaged axial particle velocity predicted along the radial direction
by several restitution coefcients at Y 1:2 m (supercial gas velocity U g 1 m=s,
Gidaspow drag model, ke turbulent model, u 1).
Fig. 8. The time-averaged axial particle velocity predicted along the radial direction
by several specularity coefcients at Y 1:2 m (supercial gas velocity U g 1 m=s,
Gidaspow drag model, ke turbulent model, es 0:9).
1745
0
0.5
0.6
0.7
0.8
0.9
(X/D)
H=1.2 m
-1
-2
Fig. 9. Comparison of the predicted axial particle velocity with the experimental
data at Y 1:2 m and for different supercial gas velocities (a) U g 0:9 m=s and (b)
U g 1:1 m=s. (Gidaspow drag model, ke turbulent model, es 0:9, u 1).
Ug =1 m/s
YH=0.07 m
YH=0.1 m
YH=0.3 m
YH=0.5 m
YH=0.7 m
YH=1 m
YH=1.2 m
0.2
Fig. 11. The computed instantaneous solid volume fraction for different supercial
gas velocities and at t 30 s (Gidaspow drag model, ke turbulent model, es 0:9,
u 1).
0.7
0.1
0
0
0.2
0.4
0.6
0.8
(X/D)
Fig. 10. Radial distribution of the axial solid volume fraction at different axial bed
distances for U g 1 m=s. (Gidaspow drag model, ke turbulent model, es 0:9,
u 1).
0.3
0.6
0.5
0.4
0.3
0.5
0.6
0.7
0.8
0.9
(X/D)
Fig. 12. The time-averaged standard deviation of axial particle velocity for different
supercial gas velocities along the radial direction at Y 1 m (Gidaspow drag
model, ke turbulent model, es 0:9, u 1).
region with the supercial gas velocity. Indeed, in the case of high
velocity (U g 1:1 m=s) there are more particles entrained into
the upper dilute region, as previously seen in Fig. 11. An increase
of the supercial gas velocity leads then to further bubble coalescence and to an increase of the drag forces acting on the particles.
The ow structure in the upper zone becomes then more heterogeneous, leading to increasing particles velocity uctuations.
We can also observe from Fig. 12 that the shape of the velocity
uctuations plots changes close to the wall by accusing a sudden
decrease due to the existence of a bulk annulus dense solids downward ow under all velocity cases.
1746
[13] J.L. Sinclair, R. Jackson, Gasparticle ow in a vertical pipe with particleparticle interactions, AIChE J. 35 (1989) 14731496.
[14] D. Gidaspow, Multiphase Flow Fluidization: Continuum Kinetic Theory
Description, Academic Press, Boston, 1994.
[15] C. Pain, S. Mansoorzadeh, C.R.E.D. Oliveira, A.J.H. Goddard, Numerical
modeling of gassolid uidized beds using the two-uid approach, Int. J.
Numer. Meth. Fluids 36 (2001) 91124.
[16] F. Taghipour, N. Ellis, C. Wong, Experimental and computational study of gas
solid uidized bed hydrodynamics, Chem. Eng. Sci. J. 60 (2005) 68576867.
[17] M. Syamlal, T.J. OBrien, Computer simulation of bubbles in a uidized bed,
AIChE Symp. Ser. 85 (1989) 2231.
[18] C.Y. Wen, Y.H. Yu, Mechanics of uidization, Chem. Eng. Progr. Symp. Ser. 62
(1966) 100111.
[19] D. Geldart, The effect of particle size and size distribution on the behavior of
gas-uidized bed, Powder Technol. 6 (1972) 201215.
[20] H. Qi, C. You, A. Boemer, U. Renz, 2000. Eulerian simulation of gassolid twophase ow in a CFB-riser under consideration of cluster effects. in: D. Xu, S.
Mori (Eds.), Fluidization 2000: Science and Technology, Xian Publishing
House, Xi, pp. 231237.
[21] S. Zimmermann, F. Taghipour, CFD modeling of the hydrodynamics and
reaction kinetics of FCC uidized-bed reactors, Ind. Eng. Chem. Res. 44 (2005)
98189827.
[22] D.Z. Zhang, W.B. Vanderheyden, The effects of mesoscopic structures on the
macroscopic momentum equations for two-phase ows, Int. J. Multiph. Flow
28 (2002) 805822.
[23] M. Ye, J. Wang, M.A. Van der Hoef, J.A.M. Kuipers, Two uid modeling of
Geldart A particles in gas-uidized beds, Particuology 6 (2008) 540548.
[24] T. Mckeen, T. Pugsley, Simulation and experimental validation of a freely
bubbling bed of FCC catalyst, Powder Technol. 129 (2003) 139152.
[25] L.G. Gibilaro, R. Di Felice, S.P. Waldram, P.U. Foscolo, Generalized friction factor
and drag coefcient correlations for uid-particle interactions, Chem. Eng. Sci.
40 (1985) 18171823.
[26] N. Yang, W. Wang, W. Ge, J. Li, CFD simulation of concurrent-up gassolid ow
in circulating uidized beds with structure-dependent drag coefcient, Chem.
Eng. J. 96 (2003) 7180.
[27] J. Li, M. Kwauk, Particleuid Two-phase FlowThe Energy minimization
Multi-scale Model, Metallurgy Industry Press, Beijing, 1994.
[28] F. Taghipour, N. Ellis, C. Wong, Experimental and computational study of gas
solid uidized bed hydrodynamics, Chem. Eng. Sci. 60 (2005) 68576867.
[29] X. Gao, C. Wu, Y.W. Cheng, L.J. Wang, X. Li, Experimental and numerical
investigation of solids behavior in a gassolid turbulent uidized bed, Powder
Technol. 228 (2012) 113.
[30] A. Almuttahar, F. Taghipour, Computational uid dynamics of high density
circulating uidized bed riser: study of modeling parameters, Powder Technol.
185 (2008) 1123.
[31] T. Li, J. Grace, X. Bi, Study of wall boundary condition in numerical simulations
of bubbling uidized beds, Powder Technol. J. 203 (2010) 447457.
[32] P.C. Johnson, R. Jackson, Frictionalcollisional constitutive relations for
granular materials with application to plane shearing, J. Fluid Mech. 176
(1987) 6793.
[33] C. Loha, H. Chattopadhyay, P.K. Chatterjee, 2013. Effect of coefcient of
restitution in EulerEuler CFD simulation of uidized-bed hydrodynamics,
Particuology, in press.
[34] M.T. Shah, R.P. Utikar, M.O. Tade, V.K. Pareek, Hydrodynamics of an FCC riser
using energy minimization multiscale drag model, Chem. Eng. J. 168 (2011)
812821.
[35] S. Benyahia, M. Syamlal, T.J. OBrien, Evaluation of boundary conditions used to
model dilute, turbulent gas/solids ows in a pipe, Powder Technol. 156 (2005)
6272.
[36] X. Lan, C. Xu, J. Gao, M. Al-Dahhan, Inuence of solid phase wall boundary
condition on CFD simulation of spouted bed, Chem. Eng. Sci. 69 (2012) 419
430.
[37] T. Van den Moortel, E. Azario, R. Santini, L. Tadrist, Experimental analysis of the
gasparticle ow in a circulating uidized bed using a phase Doppler particle
analyzer, Chem. Eng. Sci. 53 (1998) 18831899.
[38] A. Zaabout, H. Bournot, R. Occelli, A. Draoui, Solids behavior in dilute zone of a
CFB riser under turbulent conditions, Particuology 9 (2011) 598605.
[39] A. Zaabout, H. Bournot, R. Occelli, B. Kharbouch, Local solid particle behavior
inside the upper zone of a circulating uidized bed riser, Adv. Powder Technol.
22 (2011) 375382.
[40] D.G. Schaeffer, Instability in the evolution equations describing incompressible
granular ow, J. Different. Eq. 66 (1987) 1950.
[41] C. Lun, S. Savage, D. Jeffrey, N. Chepumiy, Kinetic theories of granular ow:
inelastic particles in coquette ow and slightly inelastic particles in a general
ow eld, J. Fluid Mech. 140 (1984) 223256.
[42] S. Ergun, Fluid ow through packed columns, Chem. Eng. Prog. 48 (1952) 89
94.
[43] T.J. OBrien, M. Syamlal, 1993. Particle cluster effects in the numerical
simulation of a circulating uidized bed. CFB-IV. Avidan AA, Ed. AIChE, New
York, pp. 430435.
[44] B.G.M. van Wachem, J.C. Schouten, R. Krishna, C.M. van den Bleek, Eulerian
simulations of bubbling behavior in gassolid uidized beds, Comput. Chem.
Eng. 22 (1998) 299366.
[45] C.L. Gomez, R.C. Silva, F.E. Milioli, Some modeling and numerical aspects of the
two-uid simulation of the gassolids ow in a CFB riser, Braz. J. Chem. Eng. 23
(4) (2006) 487496.
1747